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    職  稱: 特聘研究講座教授 系所成員: [ 專任教師 ]
    姓  名: 朱時宜
    Shih-I Chu
    學  歷: 1974年 美國哈佛大學化學物理學博士
    NTU AH: http://ah.ntu.edu.tw/web/Teacher!one.action?tid=3520
    個人網址:
    房  號: 1216
    電  話: (02) 3366-5104
    E-Mail(1): E-Mail(2):
    Research Associate, Joint Institute for Laboratory Astrophysics (JILA) (1974-76).

    J. Willard Gibbs Lecturer, Yale University (1976-78).

    Watkins Distinguished Professor (1990-present), University of Kansas.

    Director, Kansas Institute for Theoretical and Computational Science (1992-1996).

    Director, Kansas Center for Advanced Scientific Computing (1996-2006).

    Advisory Board, Institute of Physics, National Chiao-Tung University (1993-96).

    Advisory Board, Institute of Atomic and Molecular Sciences, Academia Sinica (1996-2007).

    Scientific Advisory Committee, Theoretical Physics Division, National Center for Theoretical Science, Taiwan (2001-2005).

    Director, Center for Quantum Science and Engineering(CQSE), (2009 – present).

    Editorial Board, Journal of Atomic, Molecular, and Optical Physics (2008-present).

    Associate Editor, Journal of Atomic and Molecular Sciences (2009-present).

    Editorial Board, Advances in Applied Physics, (2012 - present).
    J. Willard Gibbs Fellow (1976-78), Physics Department, Yale University.

    Alfred P. Sloan Foundation Fellow (1980-84).

    JILA Visiting Fellow (1984-85).

    John Simon Guggenheim Fellow (1987-88).

    Fellow, American Physical Society (1988-present).

    Olin Petefish Award in Basic Sciences (1988).

    Watkins Distinguished Professor (1990-present), University of Kansas.

    國立清華大學傑出校友(2005).

    中央研究院院士(2006-present).

    Fellow, The World Academy of Sciences (TWAS)
    「世界科學院」 院士 (Sept. 2012 - ).
    原子分子與強場物理, 超快光學, 化學物理, 量子計算與資訊
    Atomic, molecular, and strong-field physics, attosecond science and ultrafast technology, generalized Floquet theories,time-dependent density functional theory, chemical physics, quantum computing and quantum information, and optimal control theory.

    a) General Research Focus: Development of new theoretical formalisms and accurate and efficient large-scale computational methods for in-depth ab initio investigations of physical, chemical, and astronomical processes of current interest in science and/or technology.

    b) Recent Research Interests:

    Atomic and molecular physics in intense laser fields: Development of non-perturbative theoretical frameworks and both time-independent and time-dependent computational methods for accurate treatment of very-high-order (100th-5000thorder) multi-photon and nonlinear optical processes (such as very-high-order harmonic generation) in intense and ultrashort laser fields.

    Attosecond (10–18 sec) ultrafast science and technology

    Development of self-interaction-free time-dependent density functional theory (TDDFT) for accurate treatment of the excited-state and Rydberg-state electronic structure and time-dependent dynamics of many-electron quantum systems (atoms, molecules, clusters, quantum dots,nano-material,…).

    Development of time-dependent generalized pseudospectral and other new computational methods for high-precision numerical solution of time-dependent Schrodinger,Dirac,and Kohn-Sham equations in space and time.

    Quantum computing and quantum information.

    Coherent and optimal control of microscopic quantum dynamics.

    Quantum chaos and quantum fractals.

    Many-body resonance states.

    Atomic and molecular astrophysics.

    (1) X. M. Tong and S. I. Chu," Theoretical Study of Multiple High-Order Harmonic Generation by Intense Ultrashort Pulsed Laser Fields: A New Generalized seudospectral Time-Dependent Method", Chem. Phys. 217,119(1997).

    (2) X. M. Tong and S. I. Chu,"Time-Dependent Approach to High-Resolution Spectroscopy and Quantum Dynamics of Rydberg Atoms in Crossed Magnetic and Electric Fields," Phys. Rev. A 61, 031401 (R) (2000).

    (3) X. Chu and S. I. Chu," Self-Interaction-Free Time-Dependent Density Functional Theory for Molecular Processes in Strong Fields: High-Order Harmonic Generation of H2 in Intense Laser Fields," Phys.Rev. A63, 023411 (2001).

    (4) S. Han, Y. Yu, X. Chu, S. I. Chu, and Z. Wang,"Time-Resolved Measurement of Dissipation-Induced Decoherence in a Josephson Junction," Science 293, 1457 (2001).

    (5) X. Chu and S. I. Chu,"Optimization of High-Order Harmonic Generation by Genetic Algorithm and Wavelet Time-Frequency Analysis of Quantum Dipole Emission",Phys. Rev. A 64, 021403(R) (2001)

    (6) A. K. Roy and S. I. Chu,"Quantum Fluid Dynamics Approach for Strong Field Processes," Phys. Rev.A 65, 043402 (2002).

    (7) Y. Yu, S. Han, X. Chu, S. I. Chu, and Z. Wang,"Coherent Temporal Oscillations of Macroscopic Quantum States in a Josephson Junction," Science 296, 889 (2002).

    (8) S. I. Chu and D. Telnov, "Beyond the Floquet Theorem: Generalized Floquet Formalisms and Quasi-energy Methods for Atomic and Molecular Multiphoton Processes in Intense Laser Fields," Physics Reports 390,1-131 (2004).

    (9) C. P. Yang, S. I. Chu, and S. Han,"Quantum
    Information Transfer and Entanglement with SQUID Qubits in Cavity QED: A Dark-State Scheme with Tolerance for Nonuniform Device Parameter, " Phys. Rev. Lett.92,117902 (2004).

    (10) D. A. Telnov and S. I. Chu," Ab Initio Study of High-Order Harmonic Generation of H2+ in Intense Laser Fields: Time-Dependent Non-Hermitian Floquet Approach," Phys. Rev. A71, 013408 (2005).

    (11) S. I. Chu,"Recent Development of Self-Interaction-Free Time-Dependent Density
    Functional Theory for Non-perturbative Treatment of Atomic and Molecular Multiphoton Processes in Intense Laser Fields," J. Chem. Phys.123, 062207 (2005).

    (12) J. J. Carrera, X. M. Tong, and S. I. Chu,"Creation and Control of Single Attosecond XUV Pulse by Few-Cycle Laser Pulses ",Phys.Rev.A74,023404 (2006).

    (13) J. Heslar, J. J. Carrera, D. A. Telnov, and S. I. Chu,“High-order Harmonic Generation of Heteronuclear Diatomic Molecules in Intense Ultrashort Laser Fields: An All-electron TDDFT Study”, Int. J. Quantum Chem. 107, 3159 (2007).

    (14) J. Carrera, S.-K. Son, and S. I. Chu,“Ab Initio Theoretical Investigation of the Frequency comb Structure and Coherence in the VUV-XUV Regimes via High-order Harmonic Generation”, Phys. Rev. A 77, 031401(R) (2008).

    (15) S.-K. Son and S. I. Chu,“Many-Mode Floquet Theoretical Approach for Coherent Control of Multiphoton Dynamics Driven by Intense Frequency-Comb Laser Fields”, Phys. Rev. A77, 063406 (2008).

    (16) Z. Y. Zhou, S. I. Chu, and S. Y. Han, "Relaxation and decoherence of a resonantly driven qubit ", J. Phys. B: At. Mol. Opt. Phys. 41, 045506 (2008) .

    (17) J. J. Carrera, S.-K. Son, and S. I. Chu, "Ab initio theoretical investigation of the frequency comb structure and coherence in the vuv-xuv regimes via high-order harmonic generation", Phys. Rev. A 77, 031401(R) (2008).

    (18) S.-K. Son and S. I. Chu, " Many-mode Floquet theoretical approach for coherent control of multiphoton dynamics driven by intense frequency-comb laser fields", Phys. Rev. A 77, 063406 (2008).

    (19) S.-K. Son, S. Han, and S. I. Chu, " Floquet formulation for the investigation of multiphoton quantum interference in a superconducting qubit driven by a strong ac field", Phys. Rev. A 79, 032301 (2009).

    (20) D. A. Telnov and S. I. Chu, "Above-threshold-ionization spectra from the core region of a time-dependent wave packet: Alternative ab initio time-dependent approach", Phys. Rev. A 79, 043421 (2009).

    (21) D. A. Telnov and S. I. Chu, "Effects of electron structure and multielectron dynamical response on strong-field multiphoton ionization of diatomic molecules with arbitrary orientation: An all-electron time-dependent density-functional-theory approach", Phys. Rev. A 79, 041401(R) (2009).

    (22) J. J. Carrera and S. I. Chu, "Ab initio time-dependent density-functional-theory study of the frequency comb structure, coherence, and dephasing of multielectron systems in the vuv-xuv regimes via high-order harmonic generation", Phys. Rev. A 79, 063410 (2009).

    (23) Tak-San Ho, Shih-Han Hung, Hsing-Ta Chen, and Shih-I Chu, "Memory effect on the multiphoton coherent destruction of tunneling in the electron transport of nanoscale systems driven by a periodic field: A generalized Floquet approach", Phys. Rev. B 79, 235323 (2009).

    (24) C. Laughlin and S. I. Chu, "A highly accurate study of a helium atom under pressure", J. Phys. A: Math. Theor. 42, 265004 (2009) .

    (25) S.-K. Son and S. I. Chu, "Multi-electron effects on the orientation dependence and photoelectron angular distribution of multiphoton ionization of CO2 in strong laser fields," Phys. Rev. A 80, 011403(R) (2009).

    (26) S.-K. Son and S. I. Chu, "Theoretical study of orientation-dependent multiphoton ionization of polyatomic molecules in intense ultrashort laser fields: A new time-dependent Voronoi-cell finite difference method", Chem. Phys. 366, 91–102 (2009).

    (27) Z. Y. Zhou and S. I. Chu, "A time-dependent momentum-space density functional theoretical approach for electron transport dynamics in molecular devices, " Europhys. Lett. 88, 17008 (2009).

    (28) D. A. Telnov and Shih-I Chu, "Effects of multiple electronic shells on strong-field multiphoton ionization and high-order harmonic generation of diatomic molecules with arbitrary orientation: An all-electron time-dependent density-functional approach", Phys. Rev. A 80, 043412 (2009).

    (29) S. K. Son, D. A. Telnov, and S. I. Chu, "Probing the origin of elliptical high-harmonic generation from aligned molecules in linearly polarized laser fields," Phys. Rev. A82, 043829 (2010).

    (30) D. A. Telnov and S. I. Chu, “Time-dependent generalized pseudospectral method for accurate treatment of multiphoton processes of diatomic molecules in intense laser fields”, Comput. Phys. Comm. 182, 18-20 (2011).

    (31) T. S. Ho, H. Rabitz, and S. I. Chu, “A general formulation of monotonically convergent algorithms in the control of quantum dynamics beyond the linear dipole interaction”, Comput. Phys. Comm. 182, 14-17 (2011).

    (32) H. T. Chen, T. S. Ho, and S. I. Chu, " Exploration of the memory effect on the photon-assisted tunneling via a single quantum dot: A generalized Floquet theoretical approach,” International Journal of Modern Physics B25, 2251–2270 (2011).

    (33) Z. Y. Zhou and S. I. Chu, “Precision calculation of above-threshold multiphoton ionization in intense short-wavelength laser fields: The momentum-space approach and time-dependent generalized pseudospectral method,” Phys. Rev. A 83, 013405 (2011).

    (34) Z. Y. Zhou and S. I. Chu, “Photoionization dynamics and angular squeezing phenomenon in intense long-wavelength laser fields”, Phys. Rev. A 83, 033406 (2011).

    (35) J. Heslar, D. A. Telnov, and S.I. Chu, “High-order-harmonic generation in homonuclear and heteronuclear diatomic molecules: Exploration of multiple orbital contributions”, Phys. Rev. A 83, 043414 (2011).

    (36) D. A. Telnov and S. I. Chu, "Low-energy structure of above-threshold-ionization electron spectra: Role of the Coulomb threshold effect," Phys. Rev. A 83, 063406 (2011).

    (37)Y.J. Chen, C. Laughlin, and S.I.Chu, "Exploration of below-threshold harmonic generation mechanisms of cesium atoms in intense mid-infrared laser pulses" in Multiphoton Processes and Attosecond Physics, edited by K. Yamanouchi and K. Midorikawa, Springer Proc. in Physics 125, 79-84 (2012).

    (38)J. Heslar and S.I. Chu, "Ab Initio Precision Study of High-Lying Doubly Excited States of Helium in Static Electric Fields: Complex-Scaling Generalized Pseudospectral Method in Hyperspherical Coordinates", Phys. Rev. A 86, 032506 (2012).

    (39)F.Y. Jeng, D.A. Telnov, and S.I. Chu, "Below-threshold high-harmonic spectroscopy with aligned hydrogen molecular ions" in Multiphoton Processes and Attosecond Physics, edited by K. Yamanouchi and K. Midorikawa, Springer Proc. in Physics 125, 247-252 (2012).

    (40)P.-C. Li and S.I. Chu, "Effects of macroscopic propagation on spectra of broadband supercontinuum harmonics and isolated attosecond-pulse generation: Coherent control of the electron quantum trajectories in two-color laser fields", Phys. Rev. A 86, 013411 (2012).

    (41)H.T. Ng and S.I. Chu, "Coherent control of atomic spin currents in a double well", Phys. Rev. A 85, 023636 (2012).

    (42)D.A. Telnov, J. Heslar, and S.I. Chu, "Time-Dependent Density Functional Theoretical Methods for Many-Electron Molecular System" in Theoretical and Computational Developments in Modern Density Functional Theory, edited by Amlan K. Roy (Nova Science Publishers, Inc., Hauppauge, NY (USA), 2012), pp. 357-390 .

    (43)X. Wang, M. Chini, Q. Zhang, K. Zhao, Y. Wu, D.A. Telnov, S.I. Chu, and Z. Chang, "Mechanism of quasi-phase-matching in a dual-gas multijet array", Phys. Rev. A 86, 021802(R) (2012).

    (44)M. Chini, X. Wang, Y. Cheng, Y. Wu, D. Zhao, D.A. Telnov, S.I. Chu, and Z. Chang, "Sub-cycle Oscillations in Virtual States Brought to Light", Nature Sci. Rep. 3, 1105-1 (2013).

    (45)J. Guo, X.S. Liu, and S.I. Chu, "Exploration of nonsequential-double-ionization dynamics of Mg atoms in linearly and circularly polarized laser fields with different potentials", Phys. Rev. A 88, 023405 (2013).

    (46)J. Heslar, D.A. Telnov, and S.I. Chu, "Time-dependent density-functional theory with optimized effective potential and self-interaction correction and derivative discontinuity for the treatment of double ionization of He and Be atoms in intense laser fields", Phys. Rev. A 87, 052513 (2013).

    (47)J. Heslar, D.A. Telnov, and S.I. Chu, "Time-Dependent Density Functional Theoretical Methods for Nonperturbative Treatment of Multiphoton Processes of Many-Electron Molecular Systems in Intense Laser Fields" in Concepts and Methods in Modern Theoretical Chemistry: Statistical Mechanics Volume 2, edited by S.K. Ghosh and P.K. Chattaraj (Taylor & Francis Inc., Bosa Roca, USA, 2013), pp. 37-55.

    (48)P.-C. Li and S.I. Chu, "High-order-harmonic generation of Ar atoms in intense ultrashort laser fields: An all-electron time-dependent density-functional approach including macroscopic propagation effects", Phys. Rev. A 88, 053415 (2013).

    (49)S.L. Liao, T.S. Ho, H. Rabitz, and S.I. Chu, "Maximum attainable field-free molecular orientation of a thermal ensemble with near-single-cycle THz pulses", Phys. Rev. A 87, 013429 (2013).

    (50)M. Murakami and S.I. Chu, "Transient absorption spectra of the laser-dressed hydrogen atom", Phys. Rev. A 88, 043428 (2013).

    (51)D.A. Telnov, K.E. Sosnova, E. Rozenbaum, and S.I. Chu, "Exterior complex scaling method in time-dependent density-functional theory: Multiphoton ionization and high-order-harmonic generation of Ar atoms", Phys. Rev. A 87, 053406 (2013).

    (52)D. Zhao, F. l. Li, and S.I. Chu, "Coherent control and giant enhancement of multiphoton ionization and high-order-harmonic generation driven by intense frequency-comb laser fields: An ab initio theoretical investigation", Phys. Rev. A 87, 043407 (2013).

    (53)D. Zhao, F.-L. Li, and S.I. Chu, "Generation and coherent control of even-order harmonics driven by intense frequency-comb and cavity-mode fields inside a fsEC", J. Phys. B: At. Mol. Opt. Phys. 46, 145403 (2013).

    (54)Z.Y. Zhou and S.I. Chu, "Multiphoton above-threshold ionization in superintense free-electron x-ray laser fields: Beyond the dipole approximation", Phys. Rev. A 87, 023407 (2013).

    (55)K.N. Avanaki, D.A. Telnov, and S.I. Chu, "Above- and below-threshold high-order-harmonic generation of H2+ in intense elliptically polarized laser fields", Phys. Rev. A 90, 033425 (2014).

    (56)M. Chini, X. Wang, Y. Cheng, H. Wang, Y. Wu, E. Cunningham, P.-C. Li, J. Heslar, D.A. Telnov, S.I. Chu, and Z. Chang, "Coherent Phase-Matched VUV Generation by Field-Controlled Bound States", Nature Photonics 8, 437 (2014).

    (57)J. Heslar, D.A. Telnov, and S.I. Chu, "Self-Interaction-Free Time-Dependent Density Functional Theory for Nonperturbative Treatment of Orientation-Dependent Multiphoton Processes of Diatomic Molecular Systems in Intense Ultrashort Laser Fields", Chinese J. Phys. 52, 578 (2014) [Invited article for a special issue of Chinese Journal of Physics: Ultrafast intense laser science].

    (58)J. Heslar, D.A. Telnov, and S.I. Chu, "Subcycle dynamics of high-order-harmonic generation of He atoms excited by attosecond pulses and driven by near-infrared laser fields: A self-interaction-free time-dependent density-functional-theory approach", Phys. Rev. A 89, 052517 (2014).

    (59)T.S. Ho, H. Rabitz, and S.I. Chu, "Theoretical Foundations for Exploring Quantum Optimal Control of Molecules" in Advances in Multi-photon Processes and Spectroscopy, edited by S.H. Lin and Y. Fujimura (World Scientific Publishing Co. Pte. Ltd., Singapore, Hackensack New Jersey (USA), London (UK), 2014), vol. 22, pp. 1-58.

    (60)P.-C. Li, C. Laughlin, and S.I. Chu, "Generation of isolated sub-20-attosecond pulses from He atoms by two-color midinfrared laser fields", Phys. Rev. A 89, 023431 (2014).

    (61)P.-C. Li, Y.-L. Sheu, C. Laughlin, and S.-I. Chu, "Role of laser-driven electron-multirescattering in resonance-enhanced below-threshold harmonic generation in He atoms", Phys. Rev. A 90, 041401(R) (2014).

    (62)Y.L. Sheu, L.Y. Hsu, H.T. Wu, P. -C. Li, and S.I. Chu, "A new time-frequency method to reveal quantum dynamics of atomic hydrogen in intense laser pulses: Synchrosqueezing transform", AIP Advances 4, 117138 (2014).

    (63)D.A. Telnov, K.N. Avanaki, and S.I. Chu, "Subcycle transient structures in time-dependent multiphoton-ionization rates", Phys. Rev. A 90, 043404 (2014).

    (64)D.A. Telnov, J. Heslar, and S.I. Chu, "Effect of nuclear vibration on high-order harmonic generation of aligned H2+ molecules", Phys. Rev. A 90, 063412 (2014).

    (65)K.N. Avanaki, D.A. Telnov, H.Z. Jooya, and Shih-I Chu, "Generation of below-threshold even harmonics by a stretched H2+ molecular ion in intense linearly and circularly polarized laser fields", Phys. Rev. A 92, 063811 (2015).

    (66)Y. Chou, P.-C. Li, T.-S. Ho, and S.I. Chu, "Optimal control of high-order harmonics for the generation of an isolated ultrashort attosecond pulse with two-color midinfrared laser fields", Phys. Rev. A 91, 063408 (2015).

    (67)Y. Chou, P.-C. Li, T.S. Ho, and S.I. Chu, "Generation of an isolated few-attosecond pulse in optimized inhomogeneous two-color fields", Phys. Rev. A 92, 023423 (2015).

    (68)J. Heslar, D.A. Telnov, and S.I. Chu, "Subcycle dynamics of high-harmonic generation in valence-shell and virtual states of Ar atoms: A self-interaction-free time-dependent density-functional-theory approach", Phys. Rev. A 91, 023420 (2015).

    (69)H.Z. Jooya, D.A. Telnov, P.-C. Li, and S.I. Chu, "Exploration of the subcycle multiphoton ionization dynamics and transient electron density structures with Bohmian trajectories", Phys. Rev. A 91, 063412 (2015).

    (70)H.Z. Jooya, D.A. Telnov, P.-C. Li, and S.I. Chu, "Investigation of the characteristic properties of high-order harmonic spectrum in atoms using Bohmian trajectories", J. Phys. B 48, 195401 (2015).

    (71)P.-C. Li, Y.-L. Sheu, C. Laughlin, and S.I. Chu, "Dynamical origin of near- and below-threshold harmonic generation of Cs in an intense mid-infrared laser field", Nature Communications 6, 8178-1 (2015) [link has Supplementary Material ].

    (72)H.Z. Jooya, P.-C. Li, S.-L. Liao, and S.I. Chu, "Generation of isolated ultra-short attosecond pulses by coherent control of the population of excited states", Phys. Lett. A 380, 316 (2016).

    (73)M. Murakami and S.I. Chu, "Photoelectron momentum distributions of the hydrogen atom driven by multicycle elliptically polarized laser pulses", Phys. Rev. A 93, 023425 (2016).

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